Abstract # C-15

Dietary Modulation of Soluble Nucleotide Pools: Increased dUTP/dTTP Ratios Induce DNA Strand Breaks in Rat Liver C. D. Jackson, Constance Weis, Barbara J. Miller, and S. Jill James NCTR, FDA, Jefferson, AR

Purified diets lacking nucleic acids and/or methyl donors (folate, choline, methionine) result in increased ratios of soluble uridine/thymidine deoxyribonucleotide triphosphates (dUTP/dTTP) and delay progression of hepatocytes through S-phase of the cell cycle during liver regeneration. To determine if this is due to DNA damage, rats were fed either a purified basal methyl-deficient diet (lacking folate, methonine, and choline) or basal diet supplemented with: 1) folic acid, methionine, and choline; 2) methionine and choline; 3) yeast RNA; 4) calf thymus DNA; or 5) methionine, choline, and yeast RNA. Levels of dUTP and dTTP (HPLC analysis) and relative amounts of DNA strand breaks (ROPS asssay) were determined. There was a two-fold increase in both dUTP/dTTP ratios and DNA strand breaks in the basal diet compared to basal diet supplemented with methyl donors. Addition of RNA or DNA to the basal diet reduced both dUTP/dTTP ratios and DNA strand breaks. Linear regression analysis of the results indicated a direct correlation of dUTP/dTTP ratios with the level of DNA strand breaks (R= 0.94; p<0.006). This may partially explain the increased carcinogenicity of diets deficient in nucleic acids and/or methyl donors.